Enhanced Mass Transfer by Density-Driven Convection during CO2 Geological Storage
Release time:2020-06-17
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Indexed by:Journal Papers
First Author:Wang, Sijia
Correspondence Author:Jiang, LL; Song, YC (reprint author), Dalian Univ Technol, Key Lab Ocean Energy Utilizat & Energy Conservat, Minist Educ, Dalian 116024, Peoples R China.
Co-author:Liu, Yu,Zhao, Yuechao,Zhang, Yi,Jiang, Lanlan,Yu, Bin,Yin, Yong,Song, Yongchen
Date of Publication:2020-05-13
Journal:INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
Included Journals:SCIE
Document Type:J
Volume:59
Issue:19
Page Number:9300-9309
ISSN No.:0888-5885
Abstract:CO2 capture and storage (CCS) is an effective way to reduce greenhouse gas emissions. Density-driven background flow in some deep saline aquifers is of interest in the geoengineering field, which can enhance dissolution rates compared with the diffusion process. This study aimed to investigate the instability of dissolution-driven convection using high-resolution magnetic resonance imaging (MRI) technology under injection conditions. A detailed discussion on the instability of the displacement front is presented. As the Rayleigh number (Ra) increased, the onset time decreased, and the finger number density increased, while the finger growth velocity increased with increasing Pelet number (Pe). Moreover, increasing the injection rate is beneficial to the mass flux for the same value of Ra. The transverse dispersion coefficient (D-T)-Pe curve in the range of 2.34 < Pe < 33.09 agrees with previous studies. The results provide a theoretical basis for dissolution-driven convection in CCS projects.
Translation or Not:no