Photo-oxidation of gas-phase cyclohexane species over nanostructured TiO2 fabricated by different strategies
发表时间：2019-03-09
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- 论文类型：
- 期刊论文
- 第一作者：
- Zheng, Chunli
- 通讯作者：
- Li, XY (reprint author), Dalian Univ Technol, Sch Environm & Biol Sci & Technol, Key Lab Ind Ecol & Environm Engn, Dalian 116024, Peoples R China.
- 合写作者：
- Li, Xinyong,Zhao, Qidong,Qu, Zhenping,Quan, Xie
- 发表时间：
- 2009-06-15
- 发表刊物：
- SEPARATION AND PURIFICATION TECHNOLOGY
- 收录刊物：
- SCIE
- 文献类型：
- J
- 卷号：
- 67
- 期号：
- 3
- 页面范围：
- 326-330
- ISSN号：
- 1383-5866
- 关键字：
- Cyclohexane; Photo-oxidation; Acidification; In-situ FT-IR; Microwave irradiation
- 摘要：
- TiO2 photocatalyst Degussa P25 was modified by three methods: SO42- acidification (labeled as STH), SO42- acidification combined with microwave irradiation (labeled as STW), and microwave irradiation (labeled as WT), respectively. FT-IR and XRD were used to characterize the structural properties of these TiO2 samples, whereas surface photovoltage spectroscopy (SPS) provided important information on the photoelectric properties. The photo-oxidation of gaseous cyclohexane over P25, STH, STW and WT was monitored by in-situ infrared technology. The experimental results demonstrated that the modified TiO2 samples were more active than the original P25 and followed this order: WT > STW > STH > P25. During the photocatalytic oxidation of cyclohexane over WT, cyclohexane was mineralized into carbon dioxide and water. Moreover, CO was also produced in small amount. (C) 2009 Elsevier B.V. All rights reserved.
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